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Progress improvement of AgGaSe2 one crystal using the vertical Bridgman system with continual ampoule rotation and its characterization

102 @ 2090 nm). In addition, the compound melts congruently as well as excellent crystal expansion behaviors, and solitary crystals having a maximum dimensions of ≈seven × five × two mm³ are received. Theoretical analyses verify that the big NLO response originates from the synergistic outcomes of Hg–Se models, (PSe4) and nonbonding electrons. The results show that HPSe is a promising mid�?and much‐IR NLO material, and encourage a path to discovering new lessons of IR NLO resources which have been diverse from regular chalcopyrite products by grouping the linear, planar, and tetrahedral units.

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AgGaSe/sub two/ crystal advancement has become recognized by an improved Bridgman approach with only a one-zone vertical expansion furnace. The approach is to make the good-liquid interface transfer from the bottom…

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electronic transitions as well as band get more info gaps Eg progressively maximize since the lithium content material improves, according to

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The substitute of 50 % of the hefty Ag�?cations with light Li�?enhances the band hole to 2.2 eV (vs. one.seven eV in AgGaSe2). The LDT worth in AgLiGa2Se4 boosts 5 instances in comparison to that in AgGaSe2, although keeping a relatively big NLO susceptibility of 26 pm V⁻�? Moreover, the thermal growth coefficients in AgLiGa2Se4 are approximately two periods reduce in absolute value when compared with AgGaSe2, which is beneficial to the large crystal advancement. All these positive aspects would make AgLiGa2Se4 a completely new promising NLO crystal for mid‐IR laser applications.